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We construct an explicit and structured family of 3XOR instances which is hard for O(√{log n}) levels of the Sum-of-Squares hierarchy. In contrast to earlier constructions, which involve a random component, our systems are highly structured and can be constructed explicitly in deterministic polynomial time. Our construction is based on the high-dimensional expanders devised by Lubotzky, Samuels and Vishne, known as LSV complexes or Ramanujan complexes, and our analysis is based on two notions of expansion for these complexes: cosystolic expansion, and a local isoperimetric inequality due to Gromov. Our construction offers an interesting contrast to the recent work of Alev, Jeronimo and the last author (FOCS 2019). They showed that 3XOR instances in which the variables correspond to vertices in a high-dimensional expander are easy to solve. In contrast, in our instances the variables correspond to the edges of the complex.